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Characterization of the variability of radon 222 concentrations in water as a contribution to understanding the operation of an aquifer in a fractured base medium: example of the Ploemeur site, Morbihan

Thomas LE DRUILLENNEC, doctorate thesis of the Université de Bretagne Occidentale, Ecole doctorale des Sciences de la Matière de l'Information et de la Santé, 278p., defended on june 26, 2007

Document type > *Mémoire/HDR/Thesis

Keywords > radon

Research Unit > IRSN/DEI/SARG/LERAR

Authors > LE DRUILLENNEC Thomas

Publication Date > 26/06/2007

Summary

Heterogeneous fractured aquifers which developed in crystalline rocks, such as schist or granite, supply 20% of tap water production of Brittany. These fractured media present a large range of permeability. In these aquifers, fluid flow and transport of elements dissolved in water are strongly related on the geometry of the fractured network. Increasing the knowledge of the hydrogeological behaviour of the aquifer is fundamental for the management and the protection of the groundwater resources. Radon-222 is a radioactive noble gas produced from radium-226 further to the radioactive decay of uranium-238; it occurs naturally in ground waters and derives primarily from U-rich rocks and minerals that have been in contact with water. Radon-222 concentrations in waters are liable to provide significant and relevant information on both the geometry of a fracture network and the flow distribution. Furthermore, radon may also be used as a tracer in the aquifer of water exchanges between zones of variable permeability.
Three main results were obtained in this study:
1. An accurate characterisation of the radon concentrations in water was carried out in the Ploemeur aquifer (Brittany, France). These results highlight the variability in the spatial and vertical distributions of 222Rn activity in groundwater together with a wide range of concentrations extending from 0 to 1 500 Bq.L-1.
2. The influence of fracture aperture on radon content in groundwater has been demonstrated with the modelling of radon concentration. Indeed, the satisfactory results obtained with a simple crack model highlight that the geometry of the fracture network controls the radon activity in groundwater.
3. Thus, the results of pumping tests performed in the boreholes improved our understanding of the system. After the pumping test, an increase of the radon content in groundwater occurred and evidenced a contribution of a radon-rich water to supply the flow rate that seems to come from the low-permeability rock matrix. Indeed, a water flow seems to occur between the most permeable zones of the aquifer, made up of the main flow pathways, and the zones with low permeability,
consisted of the unfractured rock matrix and secondary fractures of lower permeability. Then, we compared the variability of radon volume activity with the evolution of the NO3-/SO42- ratio and the SF6 content of groundwater. The results obtained with these tracers seem to allow the hypothesis of a water flux from the rock matrix to the fractured network.


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