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Caractérisation des aérosols produits par interaction laser-matière


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Titre du congrès :1st workshop on the "Dust in Fusion Plasmas" Ville du congrès :Warsaw Date du congrès :08/07/2007

Type de document > *Congrès/colloque

Mots clés > ablation laser, caractérisation, mesures, nanoparticules

Unité de recherche > IRSN/DSU/SERAC/LPMA

Auteurs > DEWALLE Pascale, PONTREAU Sébastien, SORTAIS Céline, VENDEL Jacques, WEULERSSE Jean-Marc

Date de publication > 10/07/2007

Résumé

A surface decontamination process is here considered: laser ablation. The aim of this paper is to present the different techniques to perform a physical characterization of aerosols produced during the process. Two examples will be discussed: one is concerning paint stripping and the other one deals with graphite tiles ablation coming from Tokamak. The physical characterization is mainly focused on the number, the size distribution and the morphology of particles produced during laser ablation. The particle number was measured with a Condensation Particle Counter (CPC) and their size distribution with an Engine Exhaust Particle Sizer (EEPS, working range: 5.6-560 nm) and an Aerosizer (working range: 0.5-100 µm). In addition, a filtration system is used in order to collect the particles for Transmission Electronic Microscopy (TEM) analyses. For acrylic paint stripping, the experiments were carried out using a Nd:YAG laser working at 532 nm, the pulse duration was 5 ns. The repetition rate and the fluence have been varied respectively from 0.1 to 10 Hz and from 0.2 to 11 J.cm-2. The results showed that the aerosol produced during a laser shot is both composed of nanoparticles and submicronic particles. A mode around 70 nm was detected by the EEPS and another one around 717 nm by the Aerosizer. Moreover, the TEM analyses allow us to suppose that the nanoparticles would be aggregates of primary particles. The submicronic particles would be large spherical particles. For graphite tiles ablation, the experiments were carried out using an IPG laser (model YLP-1/120/20) working at 1 µm, the pulse duration was 100 ns. The energy of each pulse was fixed at 1 mJ and the repetition rate at 20 kHz. Two graphite tiles with hydrocarbon co-deposited layer on one side were studied. We studied both the front face of the tile (side “co-deposited layer”) and the back face of the tile (side “substrate”). A mode around 10 nm was detected by the EEPS for the side “substrate”. The mode for the side “layer” was located towards 60-90 nm. A second mode around 700-800 nm was observed by the Aerosizer for all the tiles at the same time on the side “layer” and on the side “substrate”. The further work will be to perform complementary chemical analyses on particles and gases and to set up in-situ optical methods to follow the stages of formation of the particles.